I am sure most people already use this but I always refer to students to the Organometallic hypertext book. It has excellent explanations of topics such as back-donation in organometallic complexes.
Early in 2009, Christopher Cummins’ group at MIT reported (in Science) the synthesis of AsP3, a compound that had never been isolated at room temperature. Later that year, a full article was published in JACS comparing the properties and reactivity of AsP3 to those of its molecular cousins, P4 and As4. The longer article is full of possibilities for discussion in inorganic chemistry courses, with topics including periodic trends, NMR, vibrational spectroscopy, electrochemistry, molecular orbital theory, and coordination chemistry.
I use these two handouts early in my inorganic course to outline how to count electrons and assign ligand types in a metal complex. I introduce it early so that I can use the terms "X" and "L" in class. I come back to it and hit it again when I do my unit on organometallics. The "ligands" handout is my interpretation of the MLH Green paper from 1995 (Green, M. L. H., J. Organometal.
This book called to me given my fascination with both origami and molecular model kits. While not a textbook in the true sense, the content of the book is pertinent to topics of molecular structure and symmetry and is therefore potentially valuable in both general and inorganic chemistry courses. In addition to the plans for constructing all the models (~125), there is a small amount of background information. Granted, many of these models could more easily be made using traditional model kits, but I had fun building them from paper.
This laboratory exercise was developed to compliment several weeks of freshmen or sophomore level quantum chemistry lecture material at our institution. The students meet in a computer lab on campus and use the software package known as GaussView.
This is a website which links to a wide variety of good quality YouTube mini-lectures on basic topics in chemistry, mathematics, physics and a variety of other sciences. Each video is about 10 minutes long and many go through example problems slowly and completely.
Molecular models and selected molecular orbital surfaces and slices were calculated with Spartan for HF, LiH, CO2, XeF2, and BF3, and the results were used by students in an in-class activity (covering several class sessions) to answer a series of questions.
http://firstyear.chem.usyd.edu.au/iChem/lewis.shtml
A set of Flash-based, interactive tools for students to construct Lewis structures for electron deficient, octet rule obeying and hypervalent MLx molecules and ions (x = 2 - 6).
The user chooses the number of electrons and bond type (single, double or triple) and is steered towards the correct stucture.
For cases where resonance structures are possible, the user must construct each form to complete the puzzle.